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For the first time, luminescence decay times characterizing the duration of phosphorescence of uranyl salts were measured by Edmond Becquerel in 1859 (Gaviola, 1926), and in the same year, Francis Perrin derived a mathematical relationship between fluorescence lifetime and molecular rotation, thereby contributing to the theoretical understanding of fluorescence lifetime (Perrin, 1926)
Finally, in 1843, Alexandre-Edmond Becquerel (18201891) described the emission of light by calcium sulfide deposited on paper when exposed to solar light beyond the violet part of the spectrum, being, therefore, the first to state that the emitted light is of longer wavelength than the incident light (Stokes, 1852